Abstract
Purpose The local dimension of toxicity effect on humans and ecosystem from chemical emissions into rural environments is currently not considered in impact characterization models underlying the Life Cycle Assessment (LCA) methodology. The aim of the present study was to understand the relevance of considering a local exposure environment for the magnitude of damage related to human toxicity and ecotoxicity impacts associated with chemical emissions into a local environment. Method Unit and realistic European emission scenarios were considered in a proposed multimedia nested box model, based on an existing framework modified with the inclusion of a local scale, and tested for ten chemicals in an illustrative case study. Results A substantial damage increase in terms of characterization factors in the proposed model was found for human health, mainly for local freshwater emissions (up to three orders of magnitude compared to emissions into continental freshwater for naphthalene) and soil emissions (up to two orders of magnitude, in particular for emissions into natural soil for 1,2-dichloroethane). Conclusions Based on our results, we suggest to use the proposed framework in LCA applications, when more specific information about the local emission environment is known. With respect to considering the local-scale, however, spatialized models might be preferable over nested box models to properly capture local phenomena in rather highly densely populated areas.