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Journal Article

Weak isotopic fractionation of dissolved O 2 during community respiration

Eyal Wurgaft; Israela Musan; Tanya Rivlin; Boaz Luz
Limnology and Oceanography · Vol. 67, Issue 8 · pp. 1794-1804 · 2022

Abstract

The isotopic composition of dissolved O 2 (δ 18 O) in aquatic environments is strongly affected by the preferential uptake of the lighter isotopologue during biological consumption processes. Numerous studies have shown that during incubation experiments, the isotopic effect of microorganism respiration ( ε organism ) is on the order of −20‰. However, studies of the co‐variations of O 2 and δ 18 O in natural environments show considerably weaker in situ fractionation ( ε app ). A possible explanation for this discrepancy is that a significant fraction of the O 2 consumption is diffusion‐limited. Although this is a generally accepted mechanism in sediments, it cannot explain the weak fractionations observed in mid‐ocean sites. Here, we analyze a time series of O 2 , δ 18 O, and auxiliary data from the northern Gulf of Aqaba (Red Sea). Although an incubation experiment showed strong fractionation against the heavy isotopologue ( ε organism = −24.5‰), the in situ ε app was only −14‰ in deep water isolated from the photic zone. We show that this result requires an additional O 2 consumption mechanism with weak fractionation, rather than mixing, and suggest that this mechanism is diffusion‐limited respiration into aggregates of organic material. We estimate that this mechanism could be responsible for 30% of the O 2 consumption in the Gulf and suggest that it may also constitute a major O 2 consumption pathway in the world's oceans.

Bibliographic Information

JournalLimnology and Oceanography
PublisherWiley
Publication Date2022-08-01
Publication Year2022
Volume67
Issue8
Pages1794-1804
Document TypeJournal Article
Print ISSN0024-3590
eISSN1939-5590
DOI10.1002/lno.12167
SubjectAquatic Science

Access Information

NARA Access Coverage1997-01-01~Current
Journal Homepagehttps://aslopubs.onlinelibrary.wiley.com/loi/19395590
Publisher PageOpen Publisher Page
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