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[FeFe] hydrogenases with modified azadithiolate bridgeheads serve as unidirectional hydrogen oxidation catalystsNARA Subscribed
Semi-synthetic [FeFe] hydrogenases hold exciting potential as tuneable artificial metalloenzymes for efficient hydrogen conversion (H 2 $$\rightleftharpoons$$ 2 H + + 2e − ). This work investigates the role of the bridgehead ligand in the [FeFe] hydrogenase active site through the study of two bridgehead-modified active-site variants (2-oxapropane 1,3-dithiolate, ODT, and propane 1,3-dithiolate, PDT). Replacing the native 2-az...
Global maps of soil temperatureNARA Subscribed
Research in global change ecology relies heavily on global climatic grids derived from estimates of air temperature in open areas at around 2 m above the ground. These climatic grids do not reflect conditions below vegetation canopies and near the ground surface, where critical ecosystem functions occur and most terrestrial species reside. Here, we provide global maps of soil temperature and bioclimatic variables at a 1‐km 2 r...
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